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XUV pump-probe experiments on diatom...

Schnorr, Kirsten.

XUV pump-probe experiments on diatomic moleculestracing the dynamics of electron rearrangement and interatomic coulombic decay /

紀錄類型:	書目-電子資源 : Monograph/item
正題名/作者:	XUV pump-probe experiments on diatomic moleculesby Kirsten Schnorr.
其他題名:	tracing the dynamics of electron rearrangement and interatomic coulombic decay /
作者:	Schnorr, Kirsten.
出版者:	Cham :Springer International Publishing :2015.
面頁冊數:	xi, 191 p. :ill. (some col.), digital ;24 cm.
Contained By:	Springer eBooks
標題:	Electrochemical analysis.
電子資源:	http://dx.doi.org/10.1007/978-3-319-12139-0
ISBN:	9783319121390 (electronic bk.)

XUV pump-probe experiments on diatomic moleculestracing the dynamics of electron rearrangement and interatomic coulombic decay /
Schnorr, Kirsten.

XUV pump-probe experiments on diatomic moleculestracing the dynamics of electron rearrangement and interatomic coulombic decay /[electronic resource] :by Kirsten Schnorr. - Cham :Springer International Publishing :2015. - xi, 191 p. :ill. (some col.), digital ;24 cm. - Springer theses,2190-5053. - Springer theses..

Introduction -- Photoionization and Interatomic Coulombic Decay -- Free-Electron Lasers -- Experimental Setup -- Data Analysis -- Ionization Dynamics of I2 in XUV and IR Laser Pulses -- ICD Lifetime in Ne2 -- Conclusions and Outlook -- Appendices.

This book explores the relaxation dynamics of inner-valence-ionized diatomic molecules on the basis of extreme-ultraviolet pump-probe experiments performed at the free-electron laser (FEL) in Hamburg. Firstly, the electron rearrangement dynamics in dissociating multiply charged iodine molecules is studied in an experiment that made it possible to access charge transfer in a thus far unexplored quasimolecular regime relevant for plasma and chemistry applications of the FEL. Secondly the lifetime of an efficient non-radiative relaxation process that occurs in weakly bound systems is measured directly for the first time in a neon dimer (Ne2). Interatomic Coulombic decay (ICD) has been identified as the dominant decay mechanism in inner-valence-ionized or excited van-der-Waals and hydrogen bonded systems, the latter being ubiquitous in all biomolecules. The role of ICD in DNA damage thus demands further investigation, e.g. with regard to applications like radiation therapy.

ISBN: 9783319121390 (electronic bk.)

Standard No.: 10.1007/978-3-319-12139-0doiSubjects--Topical Terms:

197304
Electrochemical analysis.

LC Class. No.: QD115

Dewey Class. No.: 543.4

XUV pump-probe experiments on diatomic moleculestracing the dynamics of electron rearrangement and interatomic coulombic decay /
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520 $a This book explores the relaxation dynamics of inner-valence-ionized diatomic molecules on the basis of extreme-ultraviolet pump-probe experiments performed at the free-electron laser (FEL) in Hamburg. Firstly, the electron rearrangement dynamics in dissociating multiply charged iodine molecules is studied in an experiment that made it possible to access charge transfer in a thus far unexplored quasimolecular regime relevant for plasma and chemistry applications of the FEL. Secondly the lifetime of an efficient non-radiative relaxation process that occurs in weakly bound systems is measured directly for the first time in a neon dimer (Ne2). Interatomic Coulombic decay (ICD) has been identified as the dominant decay mechanism in inner-valence-ionized or excited van-der-Waals and hydrogen bonded systems, the latter being ubiquitous in all biomolecules. The role of ICD in DNA damage thus demands further investigation, e.g. with regard to applications like radiation therapy.
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