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Tunneling in Molecular Magnets.
~
Northwestern University.
Tunneling in Molecular Magnets.
Record Type:
Electronic resources : Monograph/item
Title/Author:
Tunneling in Molecular Magnets.
Author:
Vijayaraghavan, Avinash.
Description:
153 p.
Notes:
Source: Dissertation Abstracts International, Volume: 72-07, Section: B, page: 4078.
Notes:
Adviser: Anupam Garg.
Contained By:
Dissertation Abstracts International72-07B.
Subject:
Physics, Condensed Matter.
Online resource:
http://pqdd.sinica.edu.tw/twdaoapp/servlet/advanced?query=3453449
ISBN:
9781124614571
Tunneling in Molecular Magnets.
Vijayaraghavan, Avinash.
Tunneling in Molecular Magnets.
- 153 p.
Source: Dissertation Abstracts International, Volume: 72-07, Section: B, page: 4078.
Thesis (Ph.D.)--Northwestern University, 2011.
This thesis is about the tunneling dynamics of the Fe8 molecule in the presence of an environment. Although a lot of progress has been made experimentally to determine among many things the extremely small tunnel splitting energies of this macromolecule, the question of how the environment affects the molecule has still not been properly understood.
ISBN: 9781124614571Subjects--Topical Terms:
226939
Physics, Condensed Matter.
Tunneling in Molecular Magnets.
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Tunneling in Molecular Magnets.
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153 p.
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Source: Dissertation Abstracts International, Volume: 72-07, Section: B, page: 4078.
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Adviser: Anupam Garg.
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Thesis (Ph.D.)--Northwestern University, 2011.
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This thesis is about the tunneling dynamics of the Fe8 molecule in the presence of an environment. Although a lot of progress has been made experimentally to determine among many things the extremely small tunnel splitting energies of this macromolecule, the question of how the environment affects the molecule has still not been properly understood.
520
$a
It is the purpose of this thesis to put forward a coherent model for the decoherence processes that affect the Fe8 molecule. The decoherence allows us to treat the Fe8 molecules as classical objects and we can write down rate equations that determine the relaxation dynamics of the entire Fe8 solid. The theoretical predictions are in very good agreement with Monte-Carlo simulations of spherical samples.
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We believe that the model developed can be generalized to different geometries and also improvised to tackle the different experimental protocols that have been undertaken on these macroscopic molecules.
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School code: 0163.
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http://pqdd.sinica.edu.tw/twdaoapp/servlet/advanced?query=3453449
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